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1Photocatalytic degradation of organic pollutants by MOFs based materials:A review显示文摘Metal-organic frameworks(MOFs)are currently popular porous materials with research and application value in various fields.Aiming at the application of MOFs in photocatalysis,this paper mainly reviews the main synthesis methods of MOFs and the latest research progress of MOFs-based photocatalysts to degrade organic pollutants in water,such as organic dyes,pharmaceuticals and personal care products,and other organic pollutants.The main characteristics of different synthesis methods of MOFs,the main design strategies of MOFs-based photocatalysts,and the excellent performance of photocatalytic degradation of organic pollutants are summarized.At the end of this paper,the practical application of MOFs,the current limitations of MOFs,the synthesis methods of MOFs,and the future development trend of MOFs photocatalysts are explained.Tianliang Xia Yingchao Lin Weizun Li Meiting Ju 2021Chinese Chemical Letters2021,32,10:8
2Catalog of Enhanced Geothermal Systems based on Heat Sources显示文摘It is common sense that a deeper well implies higher temperature in the exploration of deep geothermal resources, especially with hot dry rock(HDR) geothermal resources, which are generally exploited in terms of enhanced geothermal systems(EGS). However, temperature is always different even at the same depth in the upper crust due to different heat sources. This paper summarizes the heat sources and classifies them into two types and five sub-types: crustorigin(partial melting, non-magma-generated tectonic events and radiogenic heat production), and mantle-origin(magma and heat conducted from the mantle). A review of global EGS sites is presented related to the five sub-types of heat sources. According to our new catalog, 71% of EGS sites host mantle-origin heat sources. The temperature logging curves indicate that EGS sites which host mantle-origin magma heat sources have the highest temperature. Therefore, high heat flow(>100 m W/m^(2)) regions with mantle-origin magma heat sources should be highlighted for the future exploration of EGS. The principle to identify the heat source is elucidated by applying geophysical and geochemical methods including noble gas isotope geochemistry and lithospheric thermal structure analysis. This analytical work will be helpful for the future exploration and assessment of HDR geothermal resources.KONG Yanlong PAN Sheng REN Yaqian ZHANG Weizun WANG Ke JIANG Guangzheng CHENG Yuanzhi SUN Wenjie ZHANG Chao HU Shengbiao HE Lijuan 2021Acta Geologica Sinica(English Edition)2021,95,6:3
3Cellulose extraction from Zoysia japonica pretreated by alumina-doped MgO in AMIMCl显示文摘Le Liu Meiting Ju Weizun Li Yang Jiang 2014Carbohydrate Polymers2014,,:1
4Evaluation of pharmaceutical activities of G-protein coupled receptor targeted pharmaceuticals in Chinese wastewater effluent显示文摘The occurre nce of biologically active pharmaceuticals in aquatic enviro nments raised the potential risks to aquatic species.Among these marketed biological active pharmaceuticals,it has been estimated that40%of them target G-protein-coupled receptors(GPCRs).We have illustrated pharmaceutical activities of GPCR targeted pharmaceuticals in English and Japanese wastewater by the in vitro transforming growth factor-α(TGFα)shedding assay.However,as the most important producer and consumer of pharmaceuticals,the occurrence of GPCR targeted pharmaceuticals in China had remained unclear.In this study,we investigated the pharmaceutical activities of GPCR targeted pharmaceuticals in secondary effluents of Chinese wastewater treatment plants.We discovered antagonistic activities against angiotensin(AT1)receptor at up to 7.2×102 ng-valsartan-equivalent quantity/L in Chinese wastewater for the first time as well as agonistic activities against dopamine(D2)receptor.Furthermore,in parallel with the assay,we determined concentrations of GPCR targeted pharmaceuticals in target wastewater by liquid chromatography coupled with tandem mass spectrometry(LC-MS/MS).Through the comparison of predicted antagonistic activities calculated by concentrations and potency values from the assay,we found that the measured antagonistic activities against AT1 receptor from the assay were higher than the predicted AT1 activities from valsartan,irbesartan,and losartan,indicating the potential existence of other unknown AT1 antagonists in wastewater.Han Zhang Yingchao Lin Zhengyu Men Masaru Ihara Weizun Li Kai He 2020Chinese Chemical Letters2020,31,10:1
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