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| 1 | Low-overpotential electrochemical ammonia synthesis using BiOCl-modified 2D titanium carbide MXene显示文摘Electrochemical synthesis of ammonia has the advantages of low energy consumption and promising environmental protection,as compared to the traditional Haber-Bosch process.However,the commercial utilization of this novel system is limited by the low Faradaic efficiency,poor ammonia yield and high overpotential due to the strong NN bond and the dominant competing reaction of hydrogen evolution reaction(HER).Herein,a BiOCl-modified two-dimensional(2D)titanium carbide MXenes nanocomposite(BiOCl@Ti_(3)C_(2)T_(x))is proposed as a promising electrocatalyst for ambient nitrogen(N_(2))reduction reaction with excellent catalytic performance and superior long-term stability at low overpotential.In 0.1 mol/L HCl,this catalyst attains a high Faradic efficiency of 11.98%and a NH_(3)yield of 4.06μg h^(-1)cm^(-2)at-0.10 V(vs.RHE),benefiting from its strong interaction of Bi 6p band with the N 2p orbitals,combined with its large specific surface area and the facile electron transfer. | Yu Wang Munkhbayar Batmunkh Hui Mao Hui Li Baohua Jia Shuyao Wu Daliang Liu Ximing Song Ying Sun Tianyi Ma | 2022 | Chinese Chemical Letters2022，33，1： | 2 |
| 2 | Process Knowledge Verification Method Based on Petri Net 显示文摘 | Wang Daliang Zhang De-zheng Gao Li-xin Liu Jian- ming Zhang Huan-sheng | 2008 | IEEE Workshop on Knowle-dge Discovery and Data Mining2008，，： | 1 |
| 3 | Temperature Effect in (K_(0.5)Na_(0.5))_(0.2)(Sr_(0.75)Ba_(0.25))_(0.9)Nb_(2)0_(6): Cu Crystal Self-Pumped Phase-Conjugator显示文摘A reflectivity of 45%of the self-pumped phase-conjugate wave in (K_(0.5)Na_(0.5))_(0.2)(Sr_(0.75)Ba_(0.25))_(0.9)Nb_(2)0_(6)-Cn crystal at the environmental temperature T~70℃ has been obtained.The temperature effect in this kind of self-pumped phase-conjugator is studied. | XU Jingjun LIU Simin WU Yuanqing ZHANG Guangyin SUN Daliang SONG Yongyuan CHEN Huanchu | 1992 | Chinese Physics Letters1992，9，7： | 1 |
| 4 | Multi-source information fusion applied to structural damage diagnosis显示文摘 | Tao Liu AiQun Li YouLiang Ding DaLiang Zhao ZhiJun Li | 2011 | Structure and Infrastructure Engineering2011，，5： | 1 |
| 5 | Study of mechanism of flame-retardant SBS-modified asphalt显示文摘 | Liu Daliang Huang Yunyong Zheng Jianlong | 2009 | International Journal of Pavement Research and Technology2009，2，4： | 1 |
| 6 | Photorefractive Self-Bending and High-Performance KNSBN:Cu Crystal Self-Pumped Phase-Conjugator显示文摘The mechanism for the high-performance KNSBN:Cu crystal self-pumped phase-conjugator is first put forward in this letter as no-loop photorefractive self-bending succesive four-wave mixing interaction.And the photore fractive backscattering amplification was found to play a very important role in it. | ZHANG Guangyin XU Jingjun WU Yuanqing LIU Simin SUN Daliang SONG Yongyuan CHEN Huanchu | 1992 | Chinese Physics Letters1992，9，1： | 1 |
| 7 | A ca. 2.2Ga Acidic Magmatic Event at the Northern Margin of the Yangtze Craton: Evidence from U-Pb Dating and Hf Isotope Analysis of Zircons from the Kongling Complex显示文摘Objective The Yangtze craton experienced Paleoproterozoic collisional orogeny at ca.1.95–2.0 Ga and post-orogenic extensional events at ca.1.85 Ga related to amalgamation of the Columbia(Nuna)supercontinent(Zhao and Cawood,2012).A ca.2.15 Ga suprasubduction zone ophiolitic mélange was recongized in the ArcheanPaleoproterozoic Kongling Complex of the | XU Daliang WEI Yunxu PENG Lianhong DENG Xin HU Kun LIU Hao | 2018 | Acta Geologica Sinica(English Edition)2018，92，2： | 1 |
| 8 | MXene-assisted polymer coating from aqueous monomer solution towards dendrite-free zinc anodes显示文摘Coating polymer on the surface is an effective way to realize functional modification of the materials for diverse applications,which has been proved to enhance the stability of metal anodes in batteries.However,given the limited operability of coating from polymer dispersions,it is imperative to develop simple aqueous-based strategies from monomers for versatile polymer coating.Herein,a Ti_(3)C_(2)Tx MXene-assisted approach is proposed to construct polymer coating on zinc metal surfaces directly from the aqueous solution of monomers in an ice bath.By combining a doctor-blading method with spontaneous polymerization of monomers on the substrates at room temperature,a uniform,adhesive,and versatile coating layer assisted by a small amount of MXene is produced in one step.Additionally,MXene nanosheets serve as nanofillers to further enhance the mechanical strength and ionic conductivity of the polymer coating.Benefiting from good film formation and improved interfacial contact,the coated zinc anode exhibits a long cycling lifespan of over 1900 h.The assembled full cells show excellent cycling stability with a high capacity retention of 85.0%at 16 A g^(-1)over 2600 cycles.This work provides a simple and efficient way to produce polymer coatings directly from monomers,which may give new insights into design multifunctional polymer coatings for various applications. | Ning Wang Zhitan Wu Yu Long Derong Chen Chuannan Geng Xiaochen Liu Daliang Han Jing Zhang Ying Tao Quan-Hong Yang | 2022 | Journal of Energy Chemistry2022，31，10： | 0 |
| 9 | SYNTHESIS AND CHARACTERIZATION OF DI(2,4,6-TRIBROMOPHENOXY)TRIPHENYL-ANTIMONY显示文摘The synthetic method and characterization of di(2,4,6-tribromophenoxy)triphenyl antinony are reporledin this paper.This compound is prepared by reacting dihalotripheny-antimony with tribromophenol under defi-nite conditions and its yield is 70-80%.Relow 250℃,the product has good lhernal stability.It makes alavorable flame resisting effect on polyethylene.while the addition is ouly l0 Phr without using animeny1rioxide,the oxygen index of the polymer increases from 18.51o 26.5,and there are no adverse effects on themechanical properties of polyelhylene. | Shu Wanyin Liu Daliang Huang Kelong Wang Kaiyi Li Yuangao | 1992 | Transactions of Nonferrous Metals Society of China1992，2，2： | 0 |
| 10 | Binary trinuclear metal-oxo sub-nanomaterials for photocatalytic hydrogen and chlorine production from seawater显示文摘Owing to the need for regenerant and self-reduction problem,the hydrogen performance of sub-nano-sized trinuclear iron-oxo complexes is still far from satisfied with affordability and practicality.Herein,two binary photocatalytic systems based on trinuclear metal-oxo complexes have been first constructed and experimentally confirmed to be competent for seawater hydrogen evolution(715.4and271.9μmol of hydrogen can be found,respectively,after 48h).Notably,chloride ions act as the hole catcher and move into the gas phase in the stable form of chlorine.Similar to heterogeneous structures,homogeneous systemsnot only enhance the hydrogen performance while ensuring the stability of metal-oxo complexes,but also shorten the consumption of photogenerated carriers by dissolved impurities in the seawater.This new attempt of building pluralistic sub-nanometric systems may offer novel design strategies with noble-metal-free catalysts and low-cost candidates for traditional semiconductor materials in enhancing photocatalytic efficiency and performing chlorine evolution from seawater splitting. | Yang Wang Litong Shi Haijun Hu Bingzhi Qian Wei Hou Hui Li Xue Liu Daliang Liu Shuyao Wu Hongwei Huang Xi-Ming Song Yu Zhang Tianyi Ma | 2022 | SusMat2022，2，6： | 0 |
| 11 | Low-Dose Electron Microscopy Imaging of Electron Beam-Sensitive Crystalline Materials显示文摘As one of the most widely used characterization tools in materials science,(scanning)transmission electron microscopy((S)TEM)has the unique ability to directly image specimens with atomic resolution.Compared to diffraction-based techniques,the main advantage of(S)TEM imaging is that in addition to the periodic average structures of crystalline materials,it can be used to probe nonperiodic local structures such as surfaces,interfaces,dopants,and defects,which have crucial impacts on material properties.However,many crystalline materials are extremely sensitive to electron beam irradiation,which can only withstand dozens(or even fewer)of electrons per square angstrom before they undergo structural damage.Although using electron doses lower than the thresholds can in principle preserve their structures,the thus acquired images are too noisy to be useful.Consequently,high-resolution imaging of the inherent structures of such electron beam-sensitive materials using(S)TEM is a longstanding challenge.In recent years,the advances in electron detectors and image-acquisition methods have enabled high-resolution(S)TEM with ultralow electron doses,largely overcoming this challenge.A series of highly electron beam-sensitive materials that are traditionally considered impossible to be imaged with(S)TEM,including metal organic frameworks(MOFs),covalent organic frameworks(COFs),organic−inorganic hybrid halide perovskites,and supramolecular crystals,have been successfully imaged at atomic resolutions.This technological advance has greatly expanded the application range of electron microscopy.This Account focuses on our recent works pertaining to the high-resolution imaging of electron beam-sensitive materials using very low electron doses.We first explain that the use of direct-detection electron-counting(DDEC)cameras provides the hardware basis for successful low-dose high-resolution TEM(HRTEM).Subsequently,we introduce a suite of methods to address the challenges peculiar to low-dose HRTEM,including rapid search for crystal zone axes,precise alignment of the image stack,and accurate determination of the defocus value.These methods,combined with the use of a DDEC camera,ensure efficient imaging of electron beam-sensitive crystalline materials in the TEM mode.Moreover,we demonstrate that integrated differential phase contrast STEM(iDPC-STEM)is an effective method for acquiring directly interpretable atomic-resolution images under low-dose conditions.In addition,we share our views on the great potential of four-dimensional STEM(4D-STEM)in imaging highly electron beamsensitive materials and provide preliminary simulation results to demonstrate its feasibility.Finally,we discuss the significance of developing(S)TEM specimen preparation techniques applicable for sensitive materials and the advantages of using the cryogenic focused ion beam(cryo-FIB)technique for this purpose. | Jia Lv Hui Zhang Daliang Zhang Lingmei Liu Yu Han | 2022 | Accounts of Materials Research2022，3，5： | 0 |
| 12 | Chaos in an Ar^(+) Composite Resonator Laser Using KNSBN:Cu Crystal Self-Pumped Phase-Conjugator显示文摘Observation of the dynamics in a single-mode Ar^(+) composite resonator Jaser using KNSBN:Cu crystal seI-pumped phase-conjugator is reported.The e-quence of inatabiltieg occurring on gain change corresponds to the transition to chaos of the logistic equation.Period doubling route to chaos,and period-5,-3,-3×2 and-2 together with-3 windows in the chaotic range were observed.The strange attractor which is similar to that of the forced Duffing equation is obtained by reconstructing phase-space pictures of the system. | CAO Yongxing BA Enxu XU Jingjun WU Yuanqing LIU Simin ZHANG Guangyin SUN Daliang | 1991 | Chinese Physics Letters1991，8，11： | 0 |
| 13 | Growth and High Reflectivity Self-Pumped Phase Conjugate of Cu-Doped KNSBN Crystal显示文摘The Cu-doped'KNSBN crystals have been grown.The self-pumped phase conjugate mirrors of Cu-doped KNSBN crystals have been demonstrated.The phase conjugate reflectivity reaches as high as 68% for the crystal with 0.04 wt.%Cu-doped.The phase conjugate reflectivity and its response time were also measured as a function of the argon-ion laser wavelengths. | SUN Daliang SONG Yongyuan JIANG Quanzhong CHEN Huanchu XU Jingjun WU Yuanqing LIU Simin ZHANG Guangyin | 1992 | Chinese Physics Letters1992，9，3： | 0 |
| 14 | Designing ABC-6 family small pore zeolites by epitaxial growth approach显示文摘Aluminosilicate small pore zeolites belonging to ABC-6 family play crucially important roles in the high methanol conversion with the high selectivity of light olefins,gas separation and storage,and selective catalytic reduction of NO_(x).In this work,we report a general method,called the epitaxial growth approach,for designing ABC-6 family small pore zeolites.It is mainly realized through the epitaxial growth on the nonporous SOD-type zeolite in the presence of inorganic cations(Na^(+)and K^(+))combined with a variety of organic structure directing agents(OSDAs).In this case,a series of ABC-6 family small pore zeolites such as ERI-,SWY-,LEV-,AFX-,and PTT-type zeolites have been successfully synthesized within a few hours.More importantly,the advanced focused ion beam(FIB)and the low-dose high-resolution transmission electron microscopy(HRTEM)imaging technique have been utilized for unraveling the zeolite heterojunction at the atomic level during the epitaxial growth process.It turns out(222)crystallographic planes of the SOD-type zeolite substrate provide unique pre-building units,which facilitate the growth of targeted ABC-6 family small pore zeolites along its c-axis.Moreover,the morphologies of ERI-type zeolite can also be tuned through the epitaxial growth approach,achieving a longer lifetime in the methanol conversion. | Xiaohui Cui Jia Lv Chao Ma Yujiao Wang Zhenghao Jia Daliang Zhang Peng Guo Zhongmin Liu | 2024 | Chinese Chemical Letters2024，35，3： | 0 |
| 15 | Image Intensity Inversion Operation Using KNSBN:Cu Crystal Self-Pumped Phase-Conjugator显示文摘The image intensity inversion operation was succeeded by using the new type KNSBN.Cu crystal self-pumped phase-conjugate mirror.The new phase-conjugator was demonstrated to have the reguired specifications for this optical processing application. | XU Jingjun ZHANG Guangyin LIU Simin WU Yuanqing SUN Daliang SONG Yongyuan CHEN Huanchu | 1992 | Chinese Physics Letters1992，9，4： | 0 |
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