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| 1 | Applying Neural-Network-Based Machine Learning to Additive Manufacturing:Current Applications,Challenges,and Future Perspectives显示文摘Additive manufacturing(AM),also known as three-dimensional printing,is gaining increasing attention from academia and industry due to the unique advantages it has in comparison with traditional subtractive manufacturing.However,AM processing parameters are difficult to tune,since they can exert a huge impact on the printed microstructure and on the performance of the subsequent products.It is a difficult task to build a process-structure-property-performance(PSPP)relationship for AM using traditional numerical and analytical models.Today,the machine learning(ML)method has been demonstrated to be a valid way to perform complex pattern recognition and regression analysis without an explicit need to construct and solve the underlying physical models.Among ML algorithms,the neural network(NN)is the most widely used model due to the large dataset that is currently available,strong computational power,and sophisticated algorithm architecture.This paper overviews the progress of applying the NN algorithm to several aspects of the AM whole chain,including model design,in situ monitoring,and quality evaluation.Current challenges in applying NNs to AM and potential solutions for these problems are then outlined.Finally,future trends are proposed in order to provide an overall discussion of this interdisciplinary area. | Xinbo Qi Guofeng Chen Yong Li Xuan Cheng Changpeng Li | 2019 | Engineering2019，5，4： | 11 |
| 2 | Recent development of methanol electrooxidation catalysts for directmethanol fuel cell显示文摘Direct methanol fuel cells(DMFCs) are very promising power source for stationary and portable miniature electric appliances due to its high efficiency and low emissions of pollutants. As the key material, catalysts for both cathode and anode face several problems which hinder the commercialization of DMFCs.In this review, we mainly focus on anode catalysts of DMFCs. The process and mechanism of methanol electrooxidation on Pt and Pt-based catalysts in acidic medium have been introduced. The influences of size effect and morphology on electrocatalytic activity are discussed though whether there is a size effect in MOR catalyst is under debate. Besides, the non Pt catalysts are also listed to emphasize though Pt is still deemed as the indispensable element in anode catalyst of DMFCs in acidic medium. Different catalyst systems are compared to illustrate the level of research at present. Some debates need to be verified with experimental evidences. | Liyuan Gong Zhiyuan Yang Kui Li Wei Xing Changpeng Liu Junjie Ge | 2018 | Journal of Energy Chemistry2018，27，6： | 9 |
| 3 | Progress of Apple Rootstock Breeding and Its Use显示文摘Apple rootstock breeding has achieved great progress worldwide.In this review,we first summarize the rootstock breeding targets and utilization in main apple-producing countries.Furthermore,we discuss the focus and important research areas of apple rootstock breeding through five aspects:parent selection and setting of crosses,target genes and marker-assisted breeding,root configuration-guided breeding,apomictic resource utilization,and the application of genetic engineering.Finally,we propose an apple rootstock division plan for China,which has a large potential to provide guidance for apple rootstock breeding and utilization in different apple-producing areas of China. | Yi Wang Wei Li Xuefeng Xu Changpeng Qiu Ting Wu Qinping Wei Fengwang Ma Zhenhai Han | 2019 | Horticultural Plant Journal2019，5，5： | 6 |
| 4 | Quantum Algorithm Design:Techniques and Applications显示文摘In recent years, rapid developments of quantum computer are witnessed in both the hardware and the algorithm domains, making it necessary to have an updated review of some major techniques and applications in quantum algorithm design.In this survey as well as tutorial article, the authors ?rst present an overview of the development of quantum algorithms, then investigate ?ve important techniques: Quantum phase estimation, linear combination of unitaries, quantum linear solver, Grover search, and quantum walk, together with their applications in quantum state preparation, quantum machine learning, and quantum search. In the end, the authors collect some open problems in?uencing the development of future quantum algorithms. | SHAO Changpeng LI Yang LI Hongbo | 2019 | Journal of Systems Science & Complexity2019，32，1： | 5 |
| 5 | Nanocluster PtNiP supported on graphene as an efficient electrocatalyst for methanol oxidation reaction显示文摘In this study,phosphorus doped graphene supported PtNiP nanocluster electrocatalyst(PtNiP/P-graphene)was successfully prepared via a simple hypophosphite-assisted co-reduction method.The improved anchoring force and increased anchoring sites of graphene support result from phosphorus doping as well as size-confined growth effect of NaH_(2)PO_(2) leads to uniform dispersion of ultrafine PtNiP nanoclusters.Doped P also promotes the removal of CO-like intermediate by adjusting Pt electronic structure combining with alloyed Ni via electronic effects.As a result,the as-prepared PtNiP/P-graphene catalyst with more exposed active sites and optimized electronic structure of Pt alloy shows excellent electrocatalytic performances for methanol oxidation reaction(MOR)both in activity and durability in an acidic medium. | Long Yang Guoqiang Li Rongpeng Ma Shuai Hou Jinfa Chang Mingbo Ruan Wenbin Cai Zhao Jin Weilin Xu Guiling Wang Junjie Ge Changpeng Liu Wei Xing | 2021 | Nano Research2021，14，8： | 4 |
| 6 | Oxygen-vacancy-rich TiO_(2)enables highly active and durable water electrolysis of urchin-like RuO_(2)catalyst显示文摘The material innovation is prerequisite to accelerating sluggish oxygen evolution reaction(OER)kinetics,thus promoting the realization of hydrogen energy community.Herein,we develop an oxygen-vacancy-rich TiO_(2)supported RuO_(2)catalyst(RuO_(2)@r-TiO_(2))towards improved OER activity and stability.The oxygen vacancy on TiO_(2)not only supplies electrons to produce lower valence Ru,but also provides sufficient anchoring site for the deposition of RuO_(2)nanocrystal.Beyond that,it can generate strong electronic interaction between TiO_(2)and supported RuO_(2),and thereby tailors the intermediates’adsorption energy on the RuO_(2)surface.As a result,the derived RuO_(2)@r-TiO_(2)catalyst exhibits superior OER activity and stability with the overpotential of 211 mV at a current density of 10 mA cm^(−2)and negligible activity degradation after 6 h operation,outperforming the non-oxygen-vacancy counterpart(223.3 mV,12.75%activity loss)and RuO_(2)catalyst(234.6 mV,42.86%activity loss). | GAO HongMei XIAO MeiLing LI GuoQiang GAO LiQin MENG QingLei LUO ZhaoYan LUO ErGui LIU ChangPeng JIN Zhao GE JunJie XING Wei | 2022 | Science China(Technological Sciences)2022，65，10： | 3 |
| 7 | Accelerated oxygen reduction on Fe/N/C catalysts derived from precisely-designed ZIF precursors显示文摘Fe/N/C material is the most competitive alternative to precious-metal catalysts for oxygen reduction.In view of the present consensus on active centers,further effort is directed at maximizing the density of single Fe atoms.Here,the imperfections in commonly used doping strategy of Fe for the synthesis of zeolitic imidazolateframework(ZIF)-derived Fe/N/C catalysts are revealed.More importantly,a strikingly improved catalyst is obtained by a‘second pyrolysis’method and delivers a half-wave potential of 0.825 V(vs.RHE)in acidic media.The strong confinement effect of carbonaceous host accounts for the formation of dense single-atom sites and thus the high activity.Our findings will potentially facilitate future improvement of M/N/C catalysts. | Ergui Luo Chen Wang Yang Li Xian Wang Liyuan Gong Tuo Zhao Zhao Jin Junjie Ge Changpeng Liu Wei Xing | 2020 | Nano Research2020，13，9： | 2 |
| 8 | Identification of active sites and synergistic effect in multicomponent carbon-based Ru catalysts during electrocatalytic hydrogen evolution显示文摘Single atom catalysts(SACs)were reported to demonstrate exciting catalytic features for a number of reactions,including hydrogen evolution reaction(HER).However,the true role of these single atom sites in catalysts remains elusive,particularly for those prepared via pyrolysis,where the formation of active nanoparticle counterparts is often unavoidable.Here we report a Ru based catalyst(Ru embedded in N doped carbon spheres(Ru/NPCS))comprising of both Ru nanoclusters and Ru single sites,who demonstrates activity exceeding Pt catalyst and mass activity among the best of the Ru based catalysts under acidic conditions.The integration of proton exchange membrane water electrolysis with Ru/NPCS as a cathode exhibited an excellent hydrogen generation activity and extraordinary stability(during 120 h of electrolysis)with a 1/48 Ru loading(16.5μgRu·cm^(−2))of a commercial 20%Pt/C catalyst.Through precisely tailoring the dispersion status of the catalysts,we reveal that while ruthenium nanoclusters actively catalyze HER via Volmer–Tafel mechanism,the Ru SACs barely catalyze HER,with H*adsorption difficult to occur.Moreover,no synergy between Ru SACs and Ru cluster is revealed,meaning the Ru SACs act as a spectator rather than active species during H2 evolution. | Rongpeng Ma Xian Wang Xiaolong Yang Yang Li Changpeng Liu Junjie Ge Wei Xing | 2023 | Nano Research2023，16，1： | 2 |
| 9 | Effect of Mn2 + on the electrical nonlinearity of (Ni, Nb) - doped SnO2 varistors 显示文摘 | Changpeng Li Jinfeng Wang Wenbin Su | 2001 | Ceramics International2001，27，： | 1 |
| 10 | Microstructure Evolution and Grain Coarsening Behaviour During Partial Remelting of Cyclic Extrusion Compression Formed AZ61 Magnesium Alloy显示文摘The effects of CEC passes, isothermal holding time and reheating temperature on the microstructure evolution and grain coarsening behaviour of AZ61 magnesium alloy produced by the recrystallisation and partialmelting (RAP) process were investigated. Before partial remelting, as-cast AZ61 alloy was deformed by cyclic extrusion compression (CEC) with one pass and two pass at 330℃. After CEC, the microstructure consisted of unrecrystallized grains and deformed eutectic compounds. Increasing isothermal holding time resulted in the formation of spheroidal grains surrounded by liquid films. With increasing the isothermal holding time, the solid grain size increased and the degree of spheroidization was improved. With increasing the reheating temperature, namely increasing liquid fraction, the solid grain size obviously decreased during the period from 560℃ to 570℃ and then slightly increased after 570℃, while the shape factor increased monotonously. During partial remelting, increasing reheating temperature can properly short the isothermal holding time to obtain fine structure. Moreover, increasing the numbers of CEC passes could produce finer semi-solid mi- crostructure. The coarsening behavior of solid grains in the semi-solid state obeys Ostwald ripening and grain coalescence mechanisms. The coarsening rate constant, K, was 80 μm3 · s-1 for samples partially remelted at 595℃. After CEC plus partial remelting, the ideal and fine semi-solid state structure can be obtained, which was suitable for thixoforming. | Changpeng WANG Huasheng MEI Rongqiang LI Difan LI Ling WANG Jie LIU Zehui HUA Lijin ZHAO Feifei PEN Hui LI | 2013 | Acta Metallurgica Sinica(English Letters)2013，26，2： | 1 |
| 11 | Facile synthesis of ZnO nanorod arrays and hierarchical nano- structures for photocatalysis and gas sensor applications显示文摘 | Ma Shuaishuai Li Rong Lti Changpeng | 2011 | J Hazard Mater2011，192，2： | 1 |
| 12 | Nonlinear Electrical Properties of SnO_2-Li_2O-Nb_2O_5 Varistor System显示文摘The electrical properties of (Nb, Li)-doped SnO2 ceramics as a new varistor material were investigated. The sample 97.95%SnO2·0.50%Li2O·0.05%Nb2O5 (mol fraction) sintered at 1450= possess the highest density (ρ=6.77 g/cm3) and nonlinear electrical coefficient (α=11.6). The substitution of Sn4+ with Li+ increases the concentration of oxygen vacancies, together with the formation of solid solution, which will increase the sintering rate greatly and decrease the optimized sintering temperature. The substitution of Sn4+ with Li+ and the variation of temperature play very important effects on the densities, dielectric constant, nonlinear electrical properties and other characteristics of the samples. The properties of the grain boundary barrier and the microstructural characteristics were investigated to ensure the effect of the dopants and the temperature. A grain boundary defect barrier model was used to illustrate the grain boundary barriers formation in SnO2-Li2O-Nb2O5 varistors. | Changpeng LI, Jinfeng WANG, Wenbin SU, Hongcun CHEN and Wenxin WANGDepartment of Physics, Shandong University, Jinan 250100, China | 2002 | Journal of Materials Science & Technology2002，18，3： | 1 |
| 13 | Preparation and characterization of sulfonated poly(ether ether ketone ketone) proton exchange membranes for fuel cell application显示文摘 | Li Xianfeng Liu Changpeng Lu Hui | 2005 | Journal of Membrane Science2005，255，12： | 1 |
| 14 | Direct synthesis of sulfonated poly(ether ether keone keone) s (SPEEKKs) proton exchange membranes for fuel cell application显示文摘 | Li Xianfeng Liu Changpeng Lu Hui | 2005 | Polymer2005，46，15： | 1 |
| 15 | Facile synthesis of ZnO nanorod arrays and hierarchical nanostructures for photocatalysis and gas sensor applications显示文摘 | Shuaishuai Ma Rong Li Changpeng Lv Wei Xu Xinglong Gou | 2011 | Journal of Hazardous Materials2011，，2： | 1 |
| 16 | 显示文摘 | Wang Jinfeng Su Wenbin | 2001 | Physica B2001，307，： | 1 |
| 17 | 显示文摘 | Wang Jinfeng Su Wenbin | 2002 | Ceramics International2002，28，： | 1 |
| 18 | Nonlinear electrical properties of Ta-doped titania capacitor-varistor ceramics 显示文摘 | Changpeng Li Jinfeng Wang Xiaosu Wang | 2002 | Mater Chem Phys2002，74，2： | 1 |
| 19 | Polymer-chelation approach to high-performance Fe-Nx-C catalyst towards oxygen reduction reaction显示文摘Pyrolyzed Fe-Nx-C with atomically dispersed Fe-Nxsites are hailed as the most promising alternative to the noble metal Pt-based catalysts towards oxygen reduction reaction(ORR). However, the conventional micropore-confinement synthetic approach usually causes the insufficient utilization of active sites and mass transport resistance as the sites are located inside the micropore. We herein report a polymerchelation strategy to directly disperse the Fe-Nxactive sites onto the carbon surface. The N-rich monomer was in-situ polymerized on the carbon support and then chelated with Fe. The strong Fe-N chelating interaction is crucial to suppress Fe aggregation when undergoing the high-temperature pyrolysis. Due to the enriched surface sites, hierarchically porous structure and excellent conductivity of carbon support,the optimal catalyst(denoted as Fe-Nx-C@C-900) exhibits impressive ORR activity of onset and half-wave potential of 1.02 and 0.87 V, respectively, superior to the Pt/C benchmark. | Xue Wang Li Zhang Meiling Xiao Junjie Ge Wei Xing Changpeng Liu Jianbing Zhu | 2023 | Chinese Chemical Letters2023，34，4： | 1 |
| 20 | Nonlinear electrical properties of TiO2- Y2O3- Nb2O5 capacitorvaristor ceramics显示文摘 | LI Changpeng WANG Jinfeng WANG Xiaosu | 2001 | Mater Sci Eng B2001，85，： | 1 |
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