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| 1 | 溴代阻燃剂环境污染及毒性研究进展显示文摘溴代阻燃剂是普遍存在的一类环境污染物,包括多溴联苯醚、四溴双酚A、六溴环十二烷和十溴二苯乙烷等,在环境与生物体中均有检出。由于其具有环境持久性、长距离迁移性及生物富集性,对溴代阻燃剂的环境影响研究已经成为环境领域的热点之一。该文对溴代阻燃剂的来源、环境污染水平、毒理学效应进行综述,并提出了建议采取的溴代阻燃剂控制措施。 | 黄铸颖 李海燕 吴启航 Fu Jie Leung YS 朱立斌 骆展炜 陈俊 陆雅茵 黄雪夏 李淑更 耿新华 | 2014 | 环境与健康杂志2014，31，11： | 11 |
| 2 | Contamination by persistent toxic substances in surface sediment of urban rivers in Chaohu City, China显示文摘The concentration and spatial distribution of persistent toxic substances (PTS) in the river sediment in Chaohu City, China were investigated. A total of nine surface sediments were collected and the selected PTS pollutants including six heavy metals and nineteen polybrominated diphenyl ethers (PBDEs) were analyzed. The mean heavy metal concentrations (in mg/kg, dry weight) ranged within 0.18-1.53 (Hg), 50.08-200.18 (Cu), 118.70-313.65 (Zn), 50.77-310.85 (Cr), 37.12-92.72 (Pb) and 13.29-197.24 (As), and Cu, Zn and As have been regarded as the main metal pollutants. The levels of PBDEs (1.2-12.1 ng/g) and BDE-209 (2.4-30.5 ng/g) were at the middle level of the global range. BDE-209 was the predominant congener (67.0%-85.7%), which agrees with the fact that technical deca-BDE mixtures are the dominant PBDE formulation in China. The relative high level of PTS pollutants in the western part of the city is probably owing to the intensive agricultural activities and lack of sewerage system there. The ecological risk assessment with the sediment quality guidelines (SOGs) indicates that the urban river sediments in the city have been heavily contaminated by heavy metals with probable ecotoxicological impacts on freshwater organisms and the main toxic pollutants are Hg and As. The results of current study imply that the city, and perhaps many other small cities in China as well, requires immediate pollution control measures with emphasis on not only conventional organic pollutants but also on PTS such as heavy metals and PBDEs. | Feipeng Li Haiping Zhang Xiangzhou Meng Ling Chen Daqiang Yin | 2012 | Journal of Environmental Sciences2012，24，11： | 9 |
| 3 | Polybrominated diphenyl ethers in soil from three typical industrial areas in Beijing, China显示文摘Areas containing industrial facilities belonging to three diferent typical industries that may cause pollution by polybrominated diphenyl ethers(PBDEs) in Beijing, China were investigated. Specifically, the areas contained a solid waste incineration plant, a chemical factory, and a heat and power plant. Investigation of the pollution status of PBDEs in the surface soil from areas around these industries revealed the highest concentration of 42 PBDE congeners(118 ng/g, dry mass) at the solid waste incineration plant. In the other two plants, the highest concentrations were both 26 ng/g(dry mass). Among the PBDE homologues, the PBDE contamination at all sites showed similar congener compositions, with BDE 209 being the dominant congener. Our findings established the first contamination status of three typical industrial areas in Beijing. Furthermore, the total concentrations of 42 PBDE congeners tended to decrease as the distance from the investigated plants increased. Overall, these plants were identified as potential pollution sources of PBDEs in Beijing. Moreover, Pearson correlation analysis revealed that the major PBDE source in Beijing may be associated with the technical deca-BDE and penta-BDE mixture. Based on the data obtained in this preliminary investigation, further study of the potential of these sources to emit PBDEs in Beijing is warranted. | Yongfei Zhang Shan Fu Xinchun Liu Zheng Li Yuan Dong | 2013 | Journal of Environmental Sciences2013，25，12： | 7 |
| 4 | 十溴二苯乙烷在环境中的分布及毒理学研究进展显示文摘十溴二苯乙烷(Decabromodiphenyl ethane,DBDPE)是一种新型溴系阻燃剂,在国内外得到越来越广泛的应用,因此在环境中也开始被普遍检测到.研究发现,DBDPE有生物累积的潜在可能性,这不仅会威胁生态系统的安全,也将对人类健康产生潜在影响.目前,关于DBDPE的研究主要集中于其在土壤、沉积物、生物体等环境介质中的含量分析,而对其急性毒性效应与亚急性毒性效应的研究较少,毒理学研究方面更是缺乏.因此,笔者拟介绍DBDPE的来源、环境分布、生物富集及毒理学效应,并提出了今后研究的主要方向. | 金美青 陈紫涵 陈雯 周珊珊 包怡然 张栋 赵红挺 | 2016 | 环境化学2016，35，12： | 6 |
| 5 | Occurrence of emerging flame retardants from e-waste recycling activities in the northern part of Vietnam显示文摘This study investigated the contamination status of 21 emerging flame retardants(FRs)in soils(n=32)and river sediments(n=8)from an e-waste recycling(EWR)site in the northern part of Vietnam.Among analyzed FRs,higher levels of decabromodiphenyl ethane(DBDPE)(NDe4200 ng/g dw),1,2-bis-(2,4,6-tribromophenoxy)ethane(BTBPE)(NDe350 ng/g dw)and Dechlorane Plus isomers(DPs)(NDe65 ng/g dw)were found in soils near EWR workshops and open burning places.The highest concentrations of DBDPE(20 ng/g dw),BTBPE(5.7 ng/g dw)and DPs(6.7 ng/g dw)were also detected in sediments collected from the middle of the EWR site.The levels decreased concomitantly with increasing distance from the EWR site.These results indicate that these FRs were released to the surrounding environment from improper recycling activities,such as manual dismantling of devices and open burning of e-wastes.Moreover,the estimated daily intakes of those FRs via soil ingestion were approximately ten times higher for children than adults.To our knowledge,this is a first comprehensive study on characterization of soil and sediment contamination by a series of emerging FRs at an EWR site in Vietnam. | Masayuki Someya Go Suzuki Alin C.Ionas Nguyen Minh Tue Fuchao Xu Hidenori Matsukami Adrian Covaci Le Huu Tuyen Pham Hung Viet Shin Takahashi Shinsuke Tanabe Hidetaka Takigami | 2016 | Emerging Contaminants2016，2，2： | 5 |
| 6 | 环境介质中十溴二苯乙烷和1,2-双(2,4,6-三溴苯氧基)乙烷分布特征的研究进展显示文摘十溴二苯乙烷(DBDPE)和1,2-双(2,4,6-三溴苯氧基)乙烷(BTBPE)作为新型溴系阻燃剂,因具有亲脂性和持久性而易于在环境介质中累积。总结了DBDPE和BTBPE在生物和非生物环境介质中的分布特征。DBDPE和BTBPE易与固相紧密结合,土壤、污泥和粉尘中的浓度远高于其他环境介质中。DBDPE和BTBPE在生物中的分布与生物种类、器官组织等有一定关系,并且在人体母乳、血液和头发中也有检出。商业化DBDPE和BTBPE的生产和使用以及电子垃圾拆解活动是DBDPE和BTBPE在环境中的主要来源。未来需对DBDPE和BTBPE在不同环境介质中的迁移转化行为、生物效应的分子机制进一步展开研究。 | 王森 张兆祥 | 2020 | 同济大学学报(自然科学版)2020，48，3： | 4 |
| 7 | 泉州山美水库及入库河流沉积物中多溴二苯醚的时空分异和降解分析显示文摘为了解城市水源水库中多溴二苯醚(PBDEs)的时空分异和同系物的降解来源及其贡献,分析了泉州山美水库及入库河流表层沉积物中PBDEs的含量、污染程度、空间分布、水文期变化、赋存量、同系物组成及其降解来源的贡献.结果表明,入库河流沉积物中∑PBDEs中值(1072.1 ng·g^-1)是山美水库(160.4 ng·g^-1)的6.7倍,山美水库单位面积沉积物中∑PBDEs的赋存量(80.3 kg·km^-2)是太湖的6.3倍,北美五大湖的188倍,其污染程度较国内外大多数湖库更严重,且以BDE-209为主(84.5%~99.2%).水库大多数样点(r为0.564~0.994,P<0.034)及河流各点(r为0.953~1.0,P<0.000)间PBDEs组成相似度较高,入库区和入库河流样点间极显著正相关(r为0.779~0.964,P<0.005)且相关性强于其他功能区,显示入库河流是水库中PBDEs的主污染源.库尾区与入库河流相关性较低(r为0.454~0.915,P≤0.128),受九都镇影响较大.各样点∑PBDEs水文期变化较一致(r为0.617~0.714,P≤0.077),但水文期变化对∑PBDEs的影响统计不显著(P=0.178,Two-Way ANOVA),而点位变化则对∑PBDEs有极显著影响(P=0.0001),入库区和其他功能区有(近)显著差异(P为0.019~0.061),表明PBDEs在水库沉积物中的空间分布变异大于水文期变化.PBDEs自然降解从河流到入库区再到库中区逐渐增加,且各级还原脱溴速率不同,部分BDE因其继续降解速率较慢而累积.丰度比值法研究表明,低溴BDE主要源自十溴二苯醚的逐级还原脱溴自然降解.Deca-BDE降解产生的Nona-BDE约70%以上可较快降解生成Octa-BDE,BDE-208约85%源自BDE-209的降解,从Octa-BDE到Penta-BDE的降解过程中,部分Octa-BDE和Hexa-BDE同系物因降解较慢而累积,Penta-BDE到Tri-BDE降解率在70%以上. | 韩文亮 刘豫 冯凯文 | 2020 | 环境科学2020，41，10： | 4 |
| 8 | Profiling kidney microRNAs from juvenile grass carp(Ctenopharyngodon idella) after 56 days of oral exposure to decabromodiphenyl ethane显示文摘Grass carp(Ctenopharyngodon idella) is one of the most important species in China.Decabromodiphenyl ethane(DBDPE) is a brominated flame retardant that has been used widely in industry, and has been observed to accumulate in the tissues of fish from South China. Evidence has shown that DBDPE is toxic to aquatic animals, but the molecular response has been unclear. MicroRNAs(miRNAs) are small noncoding and negative regulatory RNAs that are 20–24 nucleotides in length, which are involved in a wide range of biological processes. We took advantage of deep-sequencing techniques to accurately and comprehensively profile the kidney mi RNA expression of grass carp after 8 weeks of oral exposure to DBDPE. After mapping sequencing data to the genome and Expressed Sequence Tags(ESTs) of grass carp, we identified 493 miRNAs in the sequenced grass carp samples, which included 51 new miRNAs. The results indicated that 5 miRNAs were significantly down-regulated and 36 miRNAs were significantly up-regulated(FDR < 0.001,1.5-fold change) after DBDPE exposure. Real-time quantitative PCR(RT-q PCR) was performed on 4 miRNAs from the two samples, and the sequencing and RT-q PCR data were consistent. This study provides the first comprehensive identification of grass carp miRNAs, and the first expression analysis of grass carp miRNAs following DBDPE exposure.The results indicated that miRNAs have potential for use as biomarkers. | Lian Gan Yuanyan Xiong Fang Dong Yunjiang Yu Lijuan Zhang Shunmei E. Liliu Zhou Xiaoxia Li Guocheng Hu | 2016 | Journal of Environmental Sciences2016，28，6： | 4 |
| 9 | 华中多雨人口密集型流域洪水预报显示文摘建立一个集总式水文模型,即基于蓄满产流的三水源新安江模型,模拟抚河流域1981—1995年的18次暴雨洪水过程;采用马斯京根分段连续算法计算河流洪水演算和水流过程线;然后将所有水流过程线线性叠加,确定水流和洪水过程;利用日尺度数据和洪水频率数据对模型进行参数率定。结果表明:该模型在现场洪水模拟中的平均确定系数为0.911,模型校准的平均径流深度误差为4.73%,验证的平均径流深度误差为8.21%,三水源新安江模型可以被应用于抚河流域的洪水预报工作中。该研究为我国中部多雨地区的洪水预报研究提供了有益的参考。 | 李雨桐 蔡宴朋 付强 宫兴龙 | 2021 | 南水北调与水利科技(中英文)2021，19，4： | 2 |
| 10 | 石河子市大气中多溴联苯醚的含量组成及气粒分配显示文摘在石河子市自2008年9月至2009年8月间每周采集大气样品,利用GC-MS分析其中的12种PBDEs,结果显示:石河子市大气中PBDEs的年平均浓度为118±83 pg/m3,低于我国其他较发达城市大气中PBDEs的含量.BDE-209是含量最高的单体,年平均含量占总量的65%,其次是BDE-47和BDE-99,年平均含量分别占总量的9%和7%.气-粒分配的研究结果显示,石河子市大气中PBDEs在气态和颗粒态间的分配并未达到平衡,温度是影响PBDEs在气相与颗粒相间分配的重要因素.比较而言,夏季最为接近平衡状态. | 杨萌 谢慧琴 贾宏亮 马万里 王荦 刘宪杰 李一凡 | 2013 | 内蒙古大学学报(自然科学版)2013，44，2： | 2 |
| 11 | 基于马尔可夫过程的湖泊生态需水保障不确定性研究显示文摘湖泊生态需水对维持其基本生态功能具有重要作用,保障生态需水已成为湖泊生态保护的重要组成部分。目前湖泊生态需水的保障方法都是在同一时间尺度下维持一个确定的水量,但湖泊水位是一个随机过程,其生态状况与湖泊水位波动密切相关,随着水位波动,湖泊生态系统的结构和功能在不断变化,导致其生态需水量也发生变化,只确定一个生态水量,不足以应对湖泊生态需水量未来可能出现的各种情况,也无法应对未来生态需水保障的不确定性,亟需对湖泊生态需水进行不确定性研究,以保障不同时期的生态需水量。以白洋淀为例,将其水位划分为5个区间,代表5个水位时期,再分析各时期的生态环境状况,得出每个时期有利于湖泊生物多样性的生态需水量。结果表明,白洋淀在枯水期、偏枯期、平水期、偏丰期、丰水期的生态水位分别为6.347、6.681、7.276、8.617、9.177 m。根据马尔可夫过程,利用改进加权马尔可夫链模型,计算出未来湖泊水位处于各个时期的概率,从而确定湖泊生态需水量的保障程度,并对未来生态需水保障情况进行预测。 | 何山 尹心安 李浩 张恩泽 | 2020 | 水生态学杂志2020，41，5： | 2 |
| 12 | The transfer and resulting negative effects of nano-and micro-plastics through the aquatic trophic web—A discreet threat to human health显示文摘The ubiquitous occurrence of plastic nano-and micro-particle contamination has raised concerns about its potential risks and impacts on the global environment,especially in aquatic ecosystems.Hundreds of aquatic species,from different trophic levels,have been affected by this“new”contaminant,which has been reported mainly in their digestive tracts.Consequently,current knowledge about plastic nano-and micro-particle spread and the potential impact on aquatic biota is growing rapidly.However,there is a significant lack of understanding of the trophic spread of microplastic contamination and integration of knowledge derived from laboratory assays with that from field research is difficult.Field experiments are unable to deal with differentiating between directly and indirectly ingested plastic microparticles.On the other hand,laboratory assays evaluating the influence of plastic microparticles and of their adhered or constitutive toxins on representative species cannot satisfactorily simulate the real environment.As a result,little is known about the effective transfer of plastic particles through the trophic net and the resulting human health risks.The present review seeks to gather information that can give a more accurate idea of the current situation and future challenges to be faced in mitigating the environmental and human effects of plastic particle pollution in aquatic,particularly estuarine,ecosystems. | Charles V.Neves Christine C.Gaylarde Jose Antonio Baptista Neto Khaue S.Vieira Bruno Pierri Carolina C.C.Waite Daniela C.Scott Estefan M.da Fonseca | 2022 | Water Biology and Security2022，1，4： | 1 |
| 13 | Polybrominated Diphenyl Ethers in Surface Sediment from Songhua River Basin,Northeast of China显示文摘Sixty sediment samples were collected from the main Songhua River in three years. Twelve polybrominated diphenyl ether( PBDE) congeners( BDE17,28,47,66,99,100,153,154,138,183,and BDE-209) were detected to state the pollution situation. The results showed that the total concentration of total PBDEs ranges from 0. 424 to 23. 0 ng / g dry weight,with the mean of 3. 02 ng / g,and the total PBDEs concentration is at relative low level compared with those worldwide. The congener profile showed that BDE-209 is the dominant congener that accounts for more than 80. 1% of total PBDEs in sediments,followed by BDE-47 and BDE-99. These profiles are consistent with a high consumption of Deca-BDEs for the brominated flame retardant market in China. The results of spatial and seasonal observations indicated that local sources,temperature variation, and hydrologic conditions are significant factors on PBDEs concentrations. Hazard quotients suggested that PBDEs pose no potential risk to benthic organisms in detected area at present. | Bo Meng Liyan Liu Wanli Ma Wenlong Li Weiwei Song Yifan Li | 2015 | Journal of Harbin Institute of Technology(New Series)2015，22，3： | 1 |
| 14 | 黄河干流表层水体和沉积物中PBDEs和NBFRs的分布特征显示文摘研究分析了2012年黄河干流表层水体及沉积物中10种多溴联苯醚(PBDEs)和6种新型溴代阻燃剂(NBFRs)的浓度水平及分布特征。BDE 209是主要的PBDEs同族体,其次是BDE47和BDE99。黄河水中的BDE47/BDE99与商用产品中的比例相似,然而黄河沉积物中的BDE47/BDE99与商用产品中却大有不同。对所测各PBDEs的同系物进行主成分分析后显示,黄河中PBDEs分布组成复杂,且当地的工业生产活动可能是黄河干流PBDEs积累的主要原因。黄河河水和沉积物中NBFRs检出率及其浓度水平较低,但六溴苯(HBB)在所有沉积物样品中均有检出,而且五溴甲苯(PBT)和五溴苯(PBBz)在所有的河水及沉积物样品中均有检出,这意味着黄河干流HBB、PBT和PBBz的污染十分普遍。与中国其他河流的数据相比,黄河的溴代阻燃剂(BFRs)水平较低,但是黄河经流的10个地区中,经济发达地区的BFRs浓度要显著高于欠发达区域。此外,河水中PBDEs的水平与人均工业产出存在很强的关联性,表明PBDEs的浓度与当地的经济发展水平显著相关。 | 王会霞 李珺琪 李光耀 王英 金军 | 2017 | 环境科学与技术2017，40，12： | 1 |
| 15 | 十溴联苯醚及十溴二苯乙烷的污染水平及毒性研究显示文摘十溴联苯醚(Decabromodiphenyl Ether,Deca-BDE)是一类常用的溴代阻燃剂,进入动植物和人体后产生甲状腺激素干扰毒性、神经毒性、生殖发育毒性等,影响代谢功能。作为Deca-BDE的替代物,十溴二苯乙烷(Decabromodiphenyl Ethane,DBDPE)的使用呈逐步上升趋势,对动植物及人类健康具有潜在的危害。综述了Deca-BDE及其替代物DBDPE的环境污染水平、来源构成、生态毒性效应和对人体健康的影响,为Deca-BDE及DBDPE的风险评估和环境监管提供参考。 | 柴斌 金美青 吴卫红 | 2021 | 杭州电子科技大学学报(自然科学版)2021，41，3： | 1 |
| 16 | 十溴二苯乙烷的研究进展显示文摘十溴二苯乙烷(DBDPE)是一种广泛使用的新型溴化阻燃剂(NBFR),具有渗出性低、使用体系稳定性高、敏感性强、适应性广等特点,可作为各类电器、塑料制品、纺织品及电子产品等材料的阻燃物。但DBDPE的污染持久性、生物积累性、远距离迁移性和固有毒性会对环境和人体产生危害,目前尚缺乏DPDPE系统毒理学的相关研究。通过查阅国内外DPDPE相关文献,介绍其应用及分布,分析了DBDPE对动物肝肾、甲状腺、生殖系统、心血管系统和神经系统等的毒性作用及其对细胞凋亡与细胞氧化应激等的影响,以期为DBDPE毒理学研究提供参考。 | 周淑馨 姜玟 李振民 齐凯歌 于美玲 | 2023 | 黑龙江科学2023，14，8： | 0 |
| 17 | 多溴联苯醚在中国环境介质及人体中的现状显示文摘多溴联苯醚(PBDEs)是持久性有机污染物的一种,对其引起的环境问题正成为我国环境工作者研究的一大热点。介绍了PBDEs的性质、生产状况和用途,综述了近年来国内对PBDEs的研究情况,总结了PBDEs在各种环境介质及人体内的浓度水平,分析了城市大气中PBDEs的浓度与城市人均GDP之间的关系,为我国今后更深入全面地开展PBDEs研究工作提供了参考。 | 李一凡 杨萌 贾宏亮 王荦 刘宪杰 | 2012 | 黑龙江大学自然科学学报2012，29，4： | 0 |
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